Improved optical and mechanical characteristics of multilayered Cu/TiON/CrO2 coating via heat treatment for solar absorbing applications

Authors

  • Hatem Taha Department of physics, College of Education for Pure Science Ibn-AL-Haitham, University of Baghdad, Baghdad, Iraq.
  • Sawsan Al-Azzawi Department of Physics, college of Education for Pure Science (Ibn Al-Haitham), University of Baghdad
  • M Mahbubur Rahman Department of Physics Jahangirnagar University Savar, Dhaka 1342 Bangladesh

DOI:

https://doi.org/10.30526/36.3.3108

Keywords:

TiON, Multilayer coatings, Solar selective absorbers, Absorptance, Emittance

Abstract

In the last few decades, growing interest has been shown in the development of new solar selective coatings based on transition metal nitride and/or oxinitride for solar absorbing applications. Solar thermal collectors are well thought out to be the most effective process of converting and harvesting solar radiation. In this investigation, Cu/TiON/CrO2 multilayered solar selective absorber coatings have been coated onto Al substrates using the dip-coating process followed by an annealing process at (400, 450, 500, 550, and 600 °C. The XRD analysis showed excellent crystalline quality for the prepared thin films along with enhanced surface features as proved by FESEM images, and the grains are in the range of (27–81) nm. The optical investigations revealed that the film annealed at 600 °C exhibits improved solar absorptance, thermal emittance, and solar selectivity of  ~ (90.7 %), (5.8 %) and 15.6, respectively. Also, the highest values of hardness ~ (26.8 GPa) and Young’s modulus ~ (250 GPa) were assigned for the film annealed at the highest temperature. Calculated optical band gaps of fabricated thin multilayered Cu/TiON/CrO2 films were found to be in the range of (1.8 – 2.10) eV.

References

Amri, A.; Solar absorptance of copper–cobalt oxide thin film coatings with nano-size, grain-like morphology: Optimization and synchrotron radiation XPS studies. Applied Surface Science, 2013, 275, 127-135. DOI: https://doi.org/10.1016/j.apsusc.2013.01.081

Rahman, M.M. Effects of annealing temperatures on the morphological, mechanical, surface chemical bonding, and solar selectivity properties of sputtered TiAlSiN thin films.Journal of Alloys and Compounds, 2016, 671,254-266. DOI: https://doi.org/10.1016/j.jallcom.2016.02.077

Ahmed, G.S., et al. Opto-electrical properties of p-SnSe: S/N-Si heterojunction for solar cell application. in AIP Conference Proceedings. 2020. AIP Publishing LLC.

Amri, A., et al., Tailoring the physicochemical and mechanical properties of optical copper-cobalt oxide thin films through annealing treatment. Surface and Coatings Technology, 2014, 239, 212-221. DOI: https://doi.org/10.1016/j.surfcoat.2013.11.044

Amri, A., et al., Surface structural features and optical analysis of nanostructured Cu-oxide thin film coatings coated via the sol-gel dip coating method. Ceramics International, 2019, 45(10), 12888-12894.

Al-Maiyaly, B.K.H., characterization of n-CdO: Mg/p-Si heterojunction dependence on annealing temperature. Ibn AL-Haitham Journal For Pure and Applied Science, 2017, 29(3),14-25.

Fadaam, S.A., et al. Synthesis and characterization of metastable phases of SnO and Sn3O4 thin films for solar cells applications. in Journal of Physics: Conference Series. 2021. IOP Publishing.

Sathy, T., et al., Structural, surface electronic bonding, optical, and mechanical features of sputtering deposited CrNiN coatings with Si and Al additives. Materials Chemistry and Physics, 2022, 277,125289.

Pulugurtha, S.R., et al., Mechanical and tribological properties of compositionally graded CrAlN films deposited by AC reactive magnetron sputtering. Surface and Coatings Technology, 2007, 202(4-7),1160-1166. DOI: https://doi.org/10.1016/j.surfcoat.2007.07.060

Schramke, K.S., et al., Nonthermal plasma synthesis of titanium nitride nanocrystals with plasmon resonances at near-infrared wavelengths relevant to photothermal therapy. ACS Applied Nano Materials, 2018, 1(6),2869-2876.

Liu, Y.; Wang, C. ; Y. Xue, The spectral properties and thermal stability of NbTiON solar selective absorbing coating,Solar energy materials and solar cells. 2012, 96,131-136. DOI: https://doi.org/10.1016/j.solmat.2011.09.034

Barshilia, H.C.,Growth, characterization and performance evaluation of Ti/AlTiN/AlTiON/AlTiO high temperature spectrally selective coatings for solar thermal power applications. Solar energy materials and solar cells, 2014,130,322-330. DOI: https://doi.org/10.1016/j.solmat.2014.07.037

Baron, F.A., et al., Structural, Optical, and Electronic Properties of Cu-Doped TiN x O y Grown by Ammonothermal Atomic Layer Deposition. ACS Applied Materials & Interfaces, 2021,13(27), 32531-32541.

Qi, Z., et al., A comparative study of the oxidation behavior of Cr2N and CrN coatings. Thin Solid Films, 2013,544,515-520. DOI: https://doi.org/10.1016/j.tsf.2013.01.031

Sousa, P.M., et al., Influence of growth temperature and carrier flux on the structure and transport properties of highly oriented CrO2 on Al2O3 (0001). Chemical Vapor Deposition, 2007. 13(10),537-545. DOI: https://doi.org/10.1002/cvde.200706592

Taha, H., et al., Improving the optoelectronic properties of titanium-doped indium tin oxide thin films. Semiconductor Science and Technology, 2017, 32(6),065011. DOI: https://doi.org/10.1088/1361-6641/aa6e3f

Ahmed, G.S., Structural and Optical properties of Polymers (PVA/PVP) doped with V2O5 composites films, Ibn AL-Haitham Journal For Pure and Applied Science, 2017, 30(2), 16-24.

Taha, H., et al., Sol-gel derived ITO-based bi-layer and tri-layer thin film coatings for organic solar cells applications. Applied Surface Science, 2020,530,147164.

Salman, S.H.; M.A. Sarmad; Ahmed,G.S.Study The Effect of Annealing on Structural and Optical Properties of Indium Selenide (InSe) Thin Films Prepared by Vacuum Thermal Evaporation Technique,in Journal of Physics: Conference Series. 2021. IOP Publishing.

Ibrahim, K., et al., Solar selective performance of metal nitride/oxynitride based magnetron sputtered thin film coatings: a comprehensive review, Journal of Optics. 2018. 20(3),033001. DOI: https://doi.org/10.1088/2040-8986/aaa2c5

Amri, A., et al., Optical and mechanical characterization of novel cobalt-based metal oxide thin films synthesized using sol–gel dip-coating method. Surface and Coatings Technology.2012, 207, 367-374. DOI: https://doi.org/10.1016/j.surfcoat.2012.07.028

de Oliveira, P.W.; Becker‐Willinger, C. ; Jilavi, M.H. Sol–Gel derived nanocomposites for optical applications. Advanced Engineering Materials. 2010, 12(5),349-361. DOI: https://doi.org/10.1002/adem.201000116

Jahan, N., et al., A holistic approach to optical characterizations of vacuum deposited Cu2ZnSnS4 thin film coatings for solar absorbing layers. Journal of Alloys and Compounds, 2021, 859,57830.

Taha, H., et al., Improved mechanical properties of sol-gel derived ITO thin films via Ag doping, Materials Today Communications, 2018. DOI: https://doi.org/10.1016/j.mtcomm.2017.12.009

Khudayer, I.H., et al., Investigation of the Structural, Optical and Electrical Properties of AgInSe2 Thin Films. Ibn AL-Haitham Journal For Pure and Applied Sciences, 2018, 31(1),37-49.

Al-Maiyaly, B.K., et al. Synthesis and characterization study of n-Bi2O3/p-Si heterojunction dependence on thickness. in AIP Conference Proceedings. 2018. AIP Publishing LLC. DOI: https://doi.org/10.1063/1.5039233

Taha, H., et al., Probing the effects of thermal treatment on the electronic structure and mechanical properties of Ti-doped ITO thin films, Journal of Alloys and Compounds, 2017. DOI: https://doi.org/10.1016/j.jallcom.2017.06.007

Taha, H., et al., Novel approach for fabricating transparent and conducting SWCNTs/ITO thin films for optoelectronic applications. The Journal of Physical Chemistry C. 2018, 122(5),3014-3027. DOI: https://doi.org/10.1021/acs.jpcc.7b10977

Downloads

Published

20-Jul-2023

Issue

Section

Physics

Publication Dates